Laser direct writing, a noncontact modified laser-induced forward transfer (LIFT) technique, has emerged as a promising technology for various applications from microelectronics printing to biofabrication. For it to be a viable technology, the bubble formation process during laser direct writing should be carefully examined. In this study, the bubble formation process during the laser direct writing of glycerol–water solutions has been studied using a nucleation-based phase explosion modeling approach. The effects of laser fluence and material properties of glycerol solution on the resulting bubble geometry have been examined both analytically and experimentally. Overall, a satisfactory modeling accuracy has been achieved, while the proposed modeling approach slightly underestimates the bubble diameter. Both the measured and predicted bubble diameters increase when the laser fluence increases. Interestingly, the measured and predicted diameters first decrease, then increase, and decrease again with the increase of glycerol concentration. Furthermore, it is noted that the bubble diameter is more sensitive to the laser fluence than the glycerol concentration.

References

1.
Schiele
,
N. R.
,
Corr
,
D. T.
,
Huang
,
Y.
,
Raof
,
N. A.
,
Xie
,
Y.
, and
Chrisey
,
D. B.
,
2010
, “
Laser-Based Direct-Write Techniques for Cell Printing
,”
Biofabrication
,
2
(
3
), p.
032001
.10.1088/1758-5082/2/3/032001
2.
Riggs
,
B. C.
,
Dias
,
A. D.
,
Schiele
,
N. R.
,
Cristescu
,
R.
,
Huang
,
Y.
,
Corr
,
D. T.
, and
Chrisey
,
D. B.
,
2011
, “
Matrix-Assisted Pulsed Laser Methods for Biofabrication
,”
MRS Bull.
,
36
(
12
), pp.
1043
1050
.10.1557/mrs.2011.276
3.
Ringeisen
,
B. R.
,
Pirlo
,
R. K.
,
Wu
,
P. K.
,
Boland
,
T.
,
Huang
,
Y.
,
Sun
,
W.
,
Hamid
,
Q.
, and
Chrisey
,
D. B.
,
2013
, “
Cell and Organ Printing Turns 15: Diverse Research to Commercial Transitions
,”
MRS Bull.
,
38
(
10
), pp.
834
843
.10.1557/mrs.2013.209
4.
Lin
,
Y.
,
Huang
,
Y.
, and
Chrisey
,
D. B.
,
2009
, “
Droplet Formation in Matrix-Assisted Pulsed-Laser Evaporation Direct Writing of Glycerol–Water Solution
,”
J. Appl. Phys.
,
105
(
9
), p.
093111
.10.1063/1.3116724
5.
Fabbro
,
R.
,
Fournier
,
J.
,
Ballard
,
P.
,
Devaux
,
D.
, and
Virmont
,
J.
,
1990
, “
Physical Study of Laser-Produced Plasma in Confined Geometry
,”
J. Appl. Phys.
,
68
(
2
), pp.
775
784
.10.1063/1.346783
6.
Sollier
,
A.
,
Berthe
,
L.
, and
Fabbro
,
R.
,
2001
, “
Numerical Modeling of the Transmission of Breakdown Plasma Generated in Water During Laser Shock Processing
,”
Eur. Phys. J. Appl. Phys.
,
16
(
2
), pp.
131
140
.10.1051/epjap:2001202
7.
Vogel
,
A.
,
Lorenz
,
K.
,
Horneffer
,
V.
,
Hüttmann
,
G.
,
Von Smolinski
,
D.
, and
Gebert
,
A.
,
2007
, “
Mechanisms of Laser-Induced Dissection and Transport of Histologic Specimens
,”
Biophys. J.
,
93
(
12
), pp.
4481
4500
.10.1529/biophysj.106.102277
8.
Fairand
,
B. P.
, and
Clauer
,
A. H.
,
1979
, “
Laser Generation of High-Amplitude Stress Waves in Materials
,”
J. Appl. Phys.
,
50
(
3
), pp.
1497
1502
.10.1063/1.326137
9.
Singh
,
R. K.
, and
Narayan
,
J.
,
1990
, “
Pulsed-Laser Evaporation Technique for Deposition of Thin Films: Physics and Theoretical Model
,”
Phys. Rev. B.
,
41
(
13
), pp.
8843
8859
.10.1103/PhysRevB.41.8843
10.
Salamin
,
Y. I.
,
Hu
,
S. X.
,
Hatsagortsyan
,
K. Z.
, and
Keitel
,
C. H.
,
2006
, “
Relativistic High-Power Laser–Matter Interactions
,”
Phys. Rep.
,
427
(
2
), pp.
41
155
.10.1016/j.physrep.2006.01.002
11.
Bulgakova
,
N. M.
, and
Bulgakov
,
A. V.
,
2001
, “
Pulsed Laser Ablation of Solids: Transition From Normal Vaporization to Phase Explosion
,”
Appl. Phys. A.
,
73
(
2
), pp.
199
208
.10.1007/s003390000686
12.
Lu
,
Q.
,
Mao
,
S. S.
,
Mao
,
X.
, and
Russo
,
R. E.
,
2002
, “
Delayed Phase Explosion During High-Power Nanosecond Laser Ablation of Silicon
,”
Appl. Phys. Lett.
,
80
(
17
), pp.
3072
3074
.10.1063/1.1473862
13.
Blake
,
J. R.
, and
Gibson
,
D. C.
,
1987
, “
Cavitation Bubbles Near Boundaries
,”
Annu. Rev. Fluid Mech.
,
19
(
1
), pp.
99
123
.10.1146/annurev.fl.19.010187.000531
14.
Brujan
,
E. A.
,
Nahen
,
K.
,
Schmidt
,
P.
, and
Vogel
,
A.
,
2001
, “
Dynamics of Laser-Induced Cavitation Bubbles Near an Elastic Boundary
,”
J. Fluid Mech.
,
433
(
1
), pp.
251
281
.10.1017/S0022112000003347
15.
Zwaan
,
E.
,
Le Gac
,
S.
,
Tsuji
,
K.
, and
Ohl
,
C. D.
,
2007
, “
Controlled Cavitation in Microfluidic Systems
,”
Phys. Rev. Lett.
,
98
(
25
),
p
. 254501.10.1103/PhysRevLett.98.254501
16.
Lin
,
Y.
,
Foy
,
K.
,
Huang
,
Y.
, and
Chrisey
,
D. B.
,
2008
, “
Bubble Formation Modeling in Matrix-Assisted Pulsed-Laser Evaporation Direct Write
,”
ASME
Paper No. MSEC_ICMP2008-72241, pp.
497
504
.10.1115/MSEC_ICMP2008-72241
17.
Wang
,
W.
,
Li
,
G.
, and
Huang
,
Y.
,
2009
, “
Modeling of Bubble Expansion-Induced Cell Mechanical Profile in Laser-Assisted Cell Direct Writing
,”
ASME J. Manuf. Sci. Eng.
,
131
(
5
), p.
051013
.10.1115/1.4000101
18.
Kattamis
,
N. T.
,
Brown
,
M. S.
, and
Arnold
,
C. B.
,
2011
, “
Finite Element Analysis of Blister Formation in Laser-Induced Forward Transfer
,”
J. Mater. Res.
,
26
(
18
), pp.
2438
2449
.10.1557/jmr.2011.215
19.
Vogel
,
A.
, and
Venugopalan
,
V.
,
2003
, “
Mechanisms of Pulsed Laser Ablation of Biological Tissues
,”
Chem. Rev.
,
103
(
2
), pp.
577
644
.10.1021/cr010379n
20.
Wang
,
W.
,
Lin
,
Y.
, and
Huang
,
Y.
,
2011
, “
Modeling of Thermoelastic Stress Wave in Laser-Assisted Cell Direct Writing
,”
ASME J. Manuf. Sci. Eng.
,
133
(
2
), p.
024502
.10.1115/1.4003612
21.
Kennedy
,
P. K.
,
Boppart
,
S. A.
,
Hammer
,
D. X.
,
Rockwell
,
B. A.
,
Noojin
,
G. D.
, and
Roach
,
W. P.
,
1995
, “
A First-Order Model for Computation of Laser-Induced Breakdown Thresholds in Ocular and Aqueous Media. Part II: Comparison to Experiment
,”
IEEE J. Quant. Electron.
,
31
(
12
), pp.
2250
2257
.10.1109/3.477754
22.
Vogel
,
A.
,
Noack
,
J.
,
Nahen
,
K.
,
Theisen
,
D.
,
Busch
,
S.
,
Parlitz
,
U.
, and
Birngruber
,
R.
,
1999
, “
Energy Balance of Optical Breakdown in Water at Nanosecond to Femtosecond Time Scales
,”
Appl. Phys. B.
,
68
(
2
), pp.
271
280
.10.1007/s003400050617
23.
Ringeisen
,
B. R.
,
Kim
,
H.
,
Barron
,
J. A.
,
Krizman
,
D. B.
,
Chrisey
,
D. B.
,
Jackman
,
S.
, and
Spargo
,
B. J.
,
2004
, “
Laser Printing of Pluripotent Embryonal Carcinoma Cells
,”
Tissue Eng.
,
10
(
3-4
), pp.
483
491
.10.1089/107632704323061843
24.
Miotello
,
A.
, and
Kelly
,
R.
,
1999
, “
Laser-Induced Phase Explosion: New Physical Problems When a Condensed Phase Approaches the Thermodynamic Critical Temperature
,”
Appl. Phys. A
,
69
(
1
), pp.
S67
S73
.10.1007/s003399900296
25.
Staveteig
,
P. T.
, and
Joseph
,
T. W.
Jr.
,
1996
, “
Dynamic 193-nm Optical Properties of Water
,”
Appl. Opt.
,
35
(
19
), pp.
3392
3403
.10.1364/AO.35.003392
26.
Lin
,
Y.
,
Huang
,
G.
,
Huang
,
Y.
,
Tzeng
,
T. J.
, and
Chrisey
,
D. B.
,
2010
, “
Effect of Laser Fluence in Laser-Assisted Direct Writing of Human Colon Cancer Cell
,”
Rapid Prototyping J.
,
16
(
3
), pp.
202
208
.10.1108/13552541011034870
27.
Kessler
,
W. J.
,
Carleton
,
K. L.
, and
Marinelli
,
W. J.
,
1993
, “
Absorption Coefficients for Water Vapor at 193 nm from 300 to 1073 K
,”
J. Quant. Spectrosc. Radiat. Transfer
,
50
(
1
), pp.
39
46
.10.1016/0022-4073(93)90127-4
28.
Kaplan
,
S. G.
, and
John
,
H. B.
,
2006
, “
Optical Properties of Fluids for 248 and 193 nm Immersion Photolithography
,”
Appl. Opt.
,
45
(
8
), pp.
1721
1724
.10.1364/AO.45.001721
29.
Zhang
,
Z.
,
2001
, “
Numerical Simulation of Short-Pulsed Laser Processing of Materials
,”
Numer. Heat Transfer Part A
,
40
(
5
),
pp
.497–509.10.1080/10407780152619801
30.
Georgiou
,
S.
, and
Antonis
,
K.
,
2003
, “
Laser-Induced Material Ejection From Model Molecular Solids and Liquids: Mechanisms, Implications, and Applications
,”
Chem. Rev.
,
103
(
2
), pp.
349
394
.10.1021/cr010429o
31.
Tomita
,
Y.
,
Tsubota
,
M.
, and
An-Naka
,
N.
,
2003
, “
Energy Evaluation of Cavitation Bubble Generation and Shock Wave Emission by Laser Focusing in Liquid Nitrogen
,”
J. Appl. Phys.
,
93
(
5
), pp.
3039
3048
.10.1063/1.1542669
32.
Docchio
,
F.
,
Regondi
,
P.
,
Capon
,
M. R.
, and
Mellerio
,
J.
,
1988
, “
Study of the Temporal and Spatial Dynamics of Plasmas Induced in Liquids by Nanosecond Nd: YAG Laser Pulses. 1: Analysis of the Plasma Starting Times
,”
Appl. Opt.
,
27
(
17
), pp.
3661
3668
.10.1364/AO.27.003661
33.
Noack
,
J.
, and
Vogel
,
A.
,
1999
, “
Laser-Induced Plasma Formation in Water at Nanosecond to Femtosecond Time Scales: Calculation of Thresholds, Absorption Coefficients, and Energy Density
,”
IEEE J. Quant. Electron.
,
35
(
8
), pp.
1156
1167
.10.1109/3.777215
34.
Chen
,
D.
, and
Zhang
,
Z.
,
2000
, “
Thermal Analysis of the Volume Absorber in Pulsed Excimer Laser Calorimeters
,”
Int. J. Heat Mass Transfer
,
43
(
17
), pp.
3061
3072
.10.1016/S0017-9310(99)00355-5
35.
Ready
,
J.
,
2012
,
Effects of High-Power Laser Radiation
,
Elsevier
,
New York
, pp.
67
125
.
36.
Duley
,
W. W.
,
2005
,
UV Lasers: Effects and Applications in Materials Science
,
Cambridge University Press
,
Cambridge, UK
, pp.
148
227
.
37.
Skripov
, V
. P.
,
1974
,
Metastable Liquids
,
Wiley
,
Hoboken, NJ
.
38.
Debenedetti
,
P. G.
,
1996
,
Metastable Liquids: Concepts and Principles
,
Princeton University Press
,
Princeton, NJ
, pp.
63
147
.
40.
Park
,
H. K.
,
1994
, “
Heat and Momentum Transfer on the Rapid Phase Change of Liquid Induced by Nanosecond-Pulsed Laser Irradiation
,” Ph.D. dissertation, University of California, Berkeley, CA.
41.
Xu
,
X.
,
2002
, “
Phase Explosion and Its Time Lag in Nanosecond Laser Ablation
,”
Appl. Surf. Sci.
,
197
, pp.
61
66
.10.1016/S0169-4332(02)00304-5
42.
Martynyuk
,
M. M.
,
1974
, “
Vaporization and Boiling of Liquid Metal in an Exploding Wire
,”
Sov. Phys. Tech. Phys.
,
19
(
6
), pp.
793
797
.
43.
Barron
,
J. A.
,
David
,
B. K.
, and
Bradley
,
R. R.
,
2005
, “
Laser Printing of Single Cells: Statistical Analysis, Cell Viability, and Stress
,”
Ann. Biomed. Eng.
,
33
(
2
), pp.
121
130
.10.1007/s10439-005-8971-x
44.
Duocastella
,
M.
,
Fernández-Pradas
,
J. M.
,
Serra
,
P.
, and
Morenza
,
J. L.
,
2008
, “
Jet Formation in the Laser Forward Transfer of Liquids
,”
Appl. Phys. A
,
93
(
2
), pp.
453
456
.10.1007/s00339-008-4781-y
45.
Yan
,
J.
,
Huang
,
Y.
,
Xu
,
C.
, and
Chrisey
,
D. B.
,
2012
, “
Effects of Fluid Properties and Laser Fluence on Jet Formation During Laser Direct Writing of Glycerol Solution
,”
J. Appl. Phys.
,
112
(
8
), p.
083105
.10.1063/1.4759344
46.
Oxtoby
,
D. W.
,
1998
, “
Nucleation of First-Order Phase Transitions
,”
Acc. Chem. Res.
,
31
(
2
), pp.
91
97
.10.1021/ar9702278
You do not currently have access to this content.