The cross-plane thermal conductivity of several nanoscale layered oxides , , and , synthesized by e-beam evaporation was measured in the range from 30 K to 300 K by the method. Thermal conductivity attains values around at room temperature in multilayer samples, formed by 20 bilayers of 10 nm , and as low as for a single bilayer. The reduction in thermal conductivity is related to the high interface density, which produces a strong barrier to heat transfer rather than to the changes of the intrinsic thermal conductivity due to the nanometer thickness of the layers. We show that the influence of the first few interfaces on the overall thermal resistance is higher than the subsequent ones. Annealing the multilayered samples to slightly increases the thermal conductivity due to changes in the microstructure. These results suggest a route to obtain suitable thermal barrier coatings for high temperature applications.
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Ultra-Low Thermal Conductivity in Nanoscale Layered Oxides
J. Alvarez-Quintana,
J. Alvarez-Quintana
Department of Physics, Nanomaterials and Microsystems Group,
Universitat Autònoma de Barcelona
, 08193 Bellaterra, Spain
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Ll. Peralba-Garcia,
Ll. Peralba-Garcia
Department of Physics, Nanomaterials and Microsystems Group,
Universitat Autònoma de Barcelona
, 08193 Bellaterra, Spain
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J. L. Lábár,
J. L. Lábár
Research Institute for Technical Physics and Materials Science
, P.O. Box 49, Budapest 114 H-1525, Hungary
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J. Rodríguez-Viejo
J. Rodríguez-Viejo
Department of Physics, Nanomaterials and Microsystems Group,
e-mail: javirod@gnam.uab.es
Universitat Autònoma de Barcelona
, 08193 Bellaterra, Spain; MATGAS Research Center, Campus Universitat Autònoma de Barcelona
, 08193 Bellaterra, Spain
Search for other works by this author on:
J. Alvarez-Quintana
Department of Physics, Nanomaterials and Microsystems Group,
Universitat Autònoma de Barcelona
, 08193 Bellaterra, Spain
Ll. Peralba-Garcia
Department of Physics, Nanomaterials and Microsystems Group,
Universitat Autònoma de Barcelona
, 08193 Bellaterra, Spain
J. L. Lábár
Research Institute for Technical Physics and Materials Science
, P.O. Box 49, Budapest 114 H-1525, Hungary
J. Rodríguez-Viejo
Department of Physics, Nanomaterials and Microsystems Group,
Universitat Autònoma de Barcelona
, 08193 Bellaterra, Spain; MATGAS Research Center, Campus Universitat Autònoma de Barcelona
, 08193 Bellaterra, Spaine-mail: javirod@gnam.uab.es
J. Heat Transfer. Mar 2010, 132(3): 032402 (6 pages)
Published Online: December 28, 2009
Article history
Received:
February 21, 2009
Revised:
July 27, 2009
Online:
December 28, 2009
Published:
December 28, 2009
Citation
Alvarez-Quintana, J., Peralba-Garcia, L., Lábár, J. L., and Rodríguez-Viejo, J. (December 28, 2009). "Ultra-Low Thermal Conductivity in Nanoscale Layered Oxides." ASME. J. Heat Transfer. March 2010; 132(3): 032402. https://doi.org/10.1115/1.4000052
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