In this work, heat transfer and phase change of an argon crystal irradiated by a picosecond pulsed laser are investigated using molecular dynamics simulations. The result reveals no clear interface when phase change occurs, but a transition region where the crystal structure and the liquid structure co-exist. Superheating is observed during the melting and vaporizing processes. The solid-liquid interface is found to move with a velocity of hundreds of meters per second, and the vapor is ejected from the surface with a vapor front velocity of hundreds of meters per second.
Issue Section:
Technical Papers
1.
Shibahara
, M.
, and Kotake
, S.
, 1997
, “Quantum Molecular Dynamics Study on Light-to-Heat Absorption Mechanism: Two Metallic Atom System
,” Int. J. Heat Mass Transf.
, 40
, pp. 3209
–3222
.2.
Shibahara
, M.
, and Kotake
, S.
, 1998
, “Quantum Molecular Dynamics Study of Light-to-Heat Absorption Mechanism in Atomic Systems
,” Int. J. Heat Mass Transf.
, 41
, pp. 839
–849
.3.
Ha¨kkinen
, H.
, and Landman
, U.
, 1993
, “Superheating, Melting, and Annealing of Copper Surfaces
,” Phys. Rev. Lett.
, 71
, pp. 1023
–1026
.4.
Anisimov
, S. I.
, Kapeliovich
, B. L.
, and Perel’man
, T. L.
, 1974
, “Electron Emission From Metal Surfaces Exposed to Ultra-short Laser Pulses
,” Sov. Phys. JETP
, 39
, pp. 375
–377
.5.
Kotake
, S.
, and Kuroki
, M.
, 1993
, “Molecular Dynamics Study of Solid Melting and Vaporization by Laser Irradiation
,” Int. J. Heat Mass Transf.
, 36
, pp. 2061
–2067
.6.
Herrmann
, R. F. W.
, and Campbell
, E. E. B.
, 1998
, “Ultrashort Pulse Laser Ablation of Silicon: an MD Simulation Study
,” Applied Physics A
, 66
, pp. 35
–42
.7.
Zhigilei
, L. V.
, Kodali
, P. B. S.
, and Garrison
, J.
, 1997
, “Molecular Dynamics Model for Laser Ablation and Desorption of Organic Solids
,” J. Phys. Chem. B
, 101
, pp. 2028
–2037
.8.
Zhigilei
, L. V.
, Kodali
, P. B. S.
, and Garrison
, J.
, 1998
, “A Microscopic View of Laser Ablation
,” J. Phys. Chem. B
, 102
, pp. 2845
–2853
.9.
Ohmura, E., Fukumoto, I., and Miyamoto, I., 1999, “Modified Molecular Dynamics Simulation on Ultrafast Laser Ablation of Metal,” Proceedings of the International Congress on Applications of Lasers and Electro-Optics, Laser Institute of America, Orlando, pp. 219–228.
10.
Girifalco
, L. A.
and Weizer
, V. G.
, 1959
, “Application of the Morse Potential Function to Cubic Metals
,” Phys. Rev.
, 114
, pp. 687
–690
.11.
Etcheverry
, J. I.
, and Mesaros
, M.
, 1999
, “Molecular Dynamics Simulation of the Production of Acoustic Waves by Pulsed Laser Irradiation
,” Phys. Rev. B
, 60
, pp. 9430
–9434
.12.
Allen, M. P., and Tildesley, D. J., 1987, Computer Simulation of Liquids, Clarendon Press, Oxford.
13.
Broughton
, J. Q.
, and Gilmer
, G. H.
, 1983
, “Molecular Dynamics Investigation of the Crystal-Fluid Interface. I. Bulk Properties
,” J. Chem. Phys.
, 79
, pp. 5095
–5104
.14.
Berendsen
, H. J. C.
, Postma
, J. P. M.
, van Gunsteren
, W. F.
, DiNola
, A.
, and Haak
, J. R.
, 1984
, “Molecular Dynamics With Coupling to an External Bath
,” J. Chem. Phys.
, 81
, pp. 3684
–90
.15.
Peterson
, O. G.
, Batchelder
, D. N.
, and Simmons
, R. O.
, 1966
, “Measurements of X-Ray Lattice Constant, Thermal Expansivity, and Isothermal Compressibility of Argon Crystals
,” Phys. Rev.
, 150
, pp. 703
–711
.16.
Wang, X., and Xu, X., 2001, “Molecular Dynamics Simulation of Thermal and Thermomechanical Phenomena in Picosecond Laser Material Interaction,” submitted to the 12th International Heat Transfer Conference.
17.
Wang, X., 2001, “Thermal and Thermomechanical Phenomena in Laser Material Interaction,” Ph.D. thesis, Purdue University, West Lafayette, IN.
18.
Chokappa
, D. K.
, Cook
, S. J.
, and Clancy
, P.
, 1989
, “Nonequilibrium Simulation Method for the Study of Directed Thermal Processing
,” Phys. Rev. B
, 39
, pp. 10075
–10087
.19.
Keeler
, G. J.
, and Batchelder
, D. N.
, 1970
, “Measurement of the Elastic Constants of Argon from 3 to 77°K
,” J. Phys. C
, 3
, pp. 510
–522
.20.
Ishizaki
, K.
, Spain
, I. L.
, and Bolsaitis
, R.
, 1975
, “Measurements of Longitudinal and Transverse Ultrasonic Wave Velocities in Compressed Solidified Argon and Their Relationship to Melting Theory
,” J. Chem. Phys.
, 63
, pp. 1401
–1410
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