Fractional Bloch equation is a generalized form of the integer order Bloch equation. It governs the dynamics of an ensemble of spins, controlling the basic process of nuclear magnetic resonance (NMR). Scale-3 (S-3) Haar wavelet operational matrix along with quasi-linearization is applied first time to detect the spin flow of fractional Bloch equations. A comparative analysis of performance of classical scale-2 (S-2) and novel scale-3 Haar wavelets (S-3 HW) has been carried out. The analysis shows that scale-3 Haar wavelets give better solutions on coarser grid point in less computation time. Error analysis shows that as we increase the level of the S-3 Haar wavelets, error goes to zero. Numerical experiments have been conducted on five test problems to illustrate the merits of the proposed novel scheme. Maximum absolute errors, comparison of exact solutions, and S-2 Haar wavelet and S-3 Haar wavelet solutions, are reported. The physical behaviors of computed solutions are also depicted graphically.

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