Overview of the U.S. Department of Energy Advanced Waste Forms Development

In order to maintain the U.S. domestic nuclear capability, its scientific technical leadership, and to keep our options open for closing the nuclear fuel cycle, the Department of Energy, Office of Nuclear Energy (DOE-NE) invests in various R&D programs to identify and resolve technical challenges related to the sustainability of the nuclear fuel cycle. Sustainable fuel cycles are those that improve uranium resource utilization, maximize energy generation, minimize waste generation, improve safety and limit proliferation risk. DOE-NE chartered a Study on the evaluation and screening of nuclear fuel cycle options, to provide information about the potential benefits and challenges of nuclear fuel cycle options and to identify a relatively small number of promising fuel cycle options with the potential for achieving substantial improvements compared to the current nuclear fuel cycle in the United States. The identification of these promising fuel cycles helps in focusing and strengthening the U.S. R&D investment needed to support the set of promising fuel cycle system options and nuclear material management approaches. DOE-NE is developing and evaluating advanced technologies for the immobilization of waste issued from aqueous and electrochemical recycling activities including off-gas treatment and advanced fuel fabrication. The long-term scope of waste form development and performance activities includes not only the development, demonstration, and technical maturation of advanced waste management concepts but also the development and parameterization of defensible models to predict the long-term performance of waste forms in geologic disposal. Along with the finding of the Evaluation and Screening Study will be presented the major research efforts that are underway for the development and demonstration of waste forms and processes including glass ceramic for high-level waste raffinate, alloy waste forms and glass ceramics composites for HLW from the electrochemical processing of fast reactor fuels, and high durability waste forms for radioiodine.