To reduce the long-term risk of the high-level liquid waste (HLLW) and the waste disposal cost, transuranium (TRU) elements should be removed from HLLW. A so-called TRPO process has been developed by Chinese scientists to partition HLLW. In this process, the extractant, trialkyl phosphine oxide (TRPO), is able to extract TRU elements into organic phase completely, which makes the treatment and disposal of raffinate HLLW much easier. However, the treatment of extracted TRU elements in organic phase, in return, becomes new troublesome issue. Generally, there are three promising ways to treat the extracted TRU elements: (1)transmutation; (2)conditioning; (3)recycling U+Pu in Purex-TRPO Integrated Process. In any of the three ways, the back extraction agents and processes play significant roles. In this paper, the investigations on back extraction agents for TRU elements, such as TTHA, DTPA, AHA, HEDPA, DOGA, and carbonates are introduced. The corresponding back extraction processes and experimental results are reviewed.
- Nuclear Engineering Division
Agents and Processes Design for TRU Elements Back Extraction in TRPO Process
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Wei, M, Liu, X, & Chen, J. "Agents and Processes Design for TRU Elements Back Extraction in TRPO Process." Proceedings of the 17th International Conference on Nuclear Engineering. Volume 5: Fuel Cycle and High and Low Level Waste Management and Decommissioning; Computational Fluid Dynamics (CFD), Neutronics Methods and Coupled Codes; Instrumentation and Control. Brussels, Belgium. July 12–16, 2009. pp. 123-130. ASME. https://doi.org/10.1115/ICONE17-75652
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