Effects of Ruthenium Release in Oxidizing Conditions on a BWR Source Term Available to Purchase

The release of ruthenium in oxygen-rich conditions from the reactor core during a severe accident may lead to formation of significantly more volatile ruthenium oxides than produced in steam atmosphere. The effect of volatile ruthenium release in a case a reference BWR nuclear plant was studied to get rough-estimates of the effects on the spreading of airborne ruthenium inside the containment and reactor building and the fission product source term. The selected accident scenario starting during shutdown conditions with pressure vessel upper head opened was a LOCA with a break in the bottom of the RPV. The results suggest that there is a remarkable amount of airborne Ru in the containment atmosphere, unlike with the standard MELCOR Ru release model which predicts no airborne Ru at all in the selected case. The total release of ruthenium from the core can be 5000 times the release predicted by the standard model. Based on the performed plant scoping studies it seems reasonable to take the release of volatile ruthenium oxides into account when assessing source terms for plants during shutdown states.